Hi, Ron,
Your Grandpa's bike is a 100 Trail. This was only built for a short period in 1968 before being suprceded by the 100 TMX. The only real differences were that the TMX had a heavy duty rear luggage rack as standard and came with full off-road "knobbly" tires, as opposed to the less extreme Trail tires on teh 100 Trail. For the purist, the 100 TMXl had silver painted headlamp shell, fork top covers and rear shock top covers. On the 100 Trail, these were all pianted in main body colour - either Candy redlike yours, or Candy Blue.
The BS100 engine was simply a BS90 Oil Injection bike with a big bore top end, so a BS90 Shop manual will serve very well for working on the engine. There is no specific manual for the BS100.
The cycle parts on the 100 trail are quite conventional so if you have some experience in working on bikes you shouldn't have too much trouble. The forks are mofified BS60 Sport, the wheels and brakes are straight BS60 Sport, the fuel tank is BS90 Sport, teh oil tank is BS175/200.
A BS90/BS100 parts manual is available for downloadng from this site, along with a BS100GP/TMX supplement which should cover all the tubular framed 100cc models.
As far as I know it was fully street legal in the States (it was never sold here in the UK, buit it is fully street legal here).
I hope that helps. Check out the pic of my TMX in the Gallery to give some idea of what the bike looks like when it's complete.
Graham Weeks.